团队介绍

能源与环境催化研究团队多年来始终致力于环境友好型催化材料的设计及其在生物质转化、有机污染物控制和清洁能源生产中的性能研究方面的工作，取得了一系列高水平和创新性的研究成果，分别在ACS Catal., Adv. Funct. Mater.、J. Catal.、Green Chem.、Appl. Catal. B: Environ.、ACS Sustainable Chem. Eng.、ACS Appl. Mater. Interfaces和Chem. Eng. J.等国际著名学术期刊发表了多篇高水平研究论文，受到了国际和国内同行的认可，并在国际学术界具有一定的影响力。

团队现有教授3人、副教授2人和师资博士后1人，团队成员先后承担多项国家自然科学基金面上和青年项目、教育部科学技术研究重大项目、教育部新世纪优秀人才支持计划项目和其它各类省部级科研和人才项目。团队曾获得教育部高等学校科学研究优秀成果奖自然科学奖二等奖和吉林省科技进步奖一等奖，获奖项目名称分别为“环境催化材料的设计及其在生物质转化和有机污染物控制中的应用”和“基于多酸的杂化催化剂的设计及其在环境催化中的应用”。团队目前的主要研究方向包括：（1）光催化环境净化和清洁能源应用研究；（2）催化转化生物质合成新一代生物油品和高附加值有机化学品研究。

Energy and environmental catalysis research team has been focusing on the design of environmentally-friendly catalytic materials for biomass transformation, organic pollutant control and clean energy production, and a series of creativity and innovation results have been achieved. The representative results have been published in the famous journals such as ACS Catal., Adv. Funct. Mater., J. Catal., Green Chem., Appl. Catal. B: Environ., ACS Sustainable Chem. Eng., ACS Appl. Mater. Interfaces and Chem. Eng. J. etc.. The work has been accepted by international and domestic peer experts, and it has some influence on the international academic fields. The members of the team have carried out more than 20 research projects, including National Natural Science Foundation of China, Key Project of Chinese Ministry of Education and the Program of New Century Excellent Talents in University. Main research interests are: (1) environmental remediation and clean energy production by photocatalysis; and (2) catalytic transformation of biomass to biofuel and value-added organics.

代表性成果

--基于g-C3N4的新型光催化材料设计及其环境净化性能研究

设计多种新颖策略，成功合成出基于g-C3N4的系列新型光催化材料。在以上材料中，通过对体相g-C3N4的电子结构和能带结构的调控，实现了显著提高g-C3N4光催化氧化水或气相中典型难降解有机污染物的总效率

--Pd单原子配位g-C3N4光催化材料设计及其清洁能源生产性能研究

结合超薄介孔g-C3N4纳米片的物理束缚作用和Pd与富含氰基的g-C3N4的配位键合作用，成功合成出层间Pd单原子配位g-C3N4光催化材料。极高的Pd原子利用率和光生电子的定向迁移的协同作用显著提高了产氢性能。

--光催化技术工程化应用探索

针对粉体光催化材料难以回收，开展了磁性功能化MOFs去除硝酸盐及有机磷农药深度去除的系列研究工作。并对光催化反应装置进行了探究，为工程化应用提供有效数据。

--固体酸催化转化生物质衍生平台化合物合成油品和有机化学品性能研究

设计多种新颖的形貌调控技术并结合化学修饰方法，制备了杂多酸、有机磺酸和酸性离子液体等功能化的硅基/碳基纳米管、纳米球和纳米孔等固体酸催化剂，成功应用于在温和条件下高活性和高选择性转化生物质衍生平台化合物合成油品和有机化学品。

代表论文

[1] Ren, M.; Zhang, X. Y.; Liu, Y. Q.; Yang, G.; Qin, L.; Meng, J. Q.; Guo, Y. H.*; Yang, Y. X.*; Interlayer palladium-single-atom-coordinated cyano-group-rich graphitic carbon nitride for enhanced photocatalytic hydrogen production performance, ACS Catal. 2022, 12, 5077-5093.

[2] Wang, X. Y.; Meng, J. Q.; Zhang, X. Y.; Liu, Y. Q.; Ren, M.; Yang, Y. X.*; Guo, Y. H.*; Controllable approach to carbon-deficient and oxygen-doped graphitic carbon nitride: robust photocatalyst against recalcitrant organic pollutants and the mechanism insight, Adv. Funct. Mater. 2021, 31, 2010763.

[3] Zhang, X. Y.; Liu, Y. Q.; Ren, M.; Yang, G.; Qin, L.; Guo, Y. H*.; Meng, J. Q.*; Precise carbon doping regulation of porous graphitic carbon nitride nanosheets enables elevated photocatalytic oxidation performance towards emerging organic pollutants, Chem. Eng. J. 2022, 433, 134551.

[4] Meng, J. Q.; Wang, X. Y.; Liu, Y. Q.; Ren, M.; Zhang, X. Y.; Ding, X. H.; Guo, Y. H.*; Yang, Y. X.*; Acid-induced molecule self-assembly synthesis of Z-scheme WO3/g-C3N4 heterojunctions for robust photocatalysis against phenolic pollutants, Chem. Eng. J. 2021, 403, 126354.

[5] Meng, J. Q.; Wang, X. Y.; Yang, X.; Hu, A. Guo, Y. H.*; Yang, Y. X.*, Enhanced gas-phase photocatalytic removal of aromatics over direct Z-scheme-dictated H3PW12O40/g-C3N4 film-coated optical fibers, Appl. Catal. B: Environ. 2019, 251, 168-180.

[6] Wang; X. Y.; Meng; J. Q.; Yang; X.; Hu; A.; Yang; Y. X.*; Guo; Y. H.*; Fabrication of a perylene tetracarboxylic diimide–graphitic carbon nitride heterojunction photocatalyst for efficient degradation of aqueous organic pollutants, ACS Appl. Mater. Interfaces 2019, 11, 588-602.

[7] Zhang, C. Y.; Pan, Y.; Guo, Y. H.*; Song, D. Y.*; Yang, Y. X.*. Supramolecular preorganization synthesis of nitrogen-doped carbon nanotubes functionalized by Brønsted acidic ionic liquid for microwave-assisted production of promising furanic derivatives, Fuel 2023, 335, 127016.

[8] Song, D. Y.*; Liu, X. F.; Khan, S.; Zhang, C. Y.; Guo, Y. H.*. Nitrogen-rich macroporous covalent triazine frameworks bearing sulfonic acid-based ionic liquids for microwave-assisted conversion of fructose to 5–hydroxymethylfurfural, Fuel 2022, 327, 125230.

[9] Sun, Y. N.; Zhang, Q. Q.; Zhang, C. Y.; Liu, J. Y.; Guo, Y. H.*; Song, D. Y.*. In situ approach to dendritic fibrous nitrogen-doped carbon nanospheres functionalized by Brønsted acidic ionic liquid and their excellent esterification catalytic performance, ACS Sustainable Chem. Eng. 2019, 7, 15114-15126.

[10] Sun, Y. N.; Zhang, Q. Q.; Zhang, P. P.; Song, D. Y.*; Guo, Y. H.*. Nitrogen-doped carbon-based acidic ionic liquid hollow nanospheres for efficient and selective conversion of fructose to 5-ethoxymethylfurfural and ethyl levulinate, ACS Sustainable Chem. Eng. 2018, 6, 6771-6782.